Ricerc@Sapienza

Femtosecond stimulated Raman scattering is a time-resolved vibrational spectroscopic technique able to access sub-picosecond dynamics and providing accurate structural information. Thanks to an appropriate combination of three laser pulses, triggering vibrational coherences delayed with respect to the photoinduced event of interest, it is capable of uncompromised temporal precision (down to 50 fs) and spectral resolution (a few wavenumbers), better than spontaneous Raman.

Illuminating a magnetic material with femtosecond laser pulses induces complex ultrafast dynamical processes. The resulting optically detectable response usually contains contributions from both the optical properties and the magnetic degrees of freedom. Disentangling all the different components concurring to the generation of the total signal is a major challenge of contemporary experimental solid-state physics.